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Flat optics nanoarrays based on few-layer MoS2 are homogeneously fabricated over large-area (cm2) transparent templates, demonstrating effective tailoring of the photon absorption in two-dimensional (2D) transition-metal dichalcogenide (TMD) layers. The subwavelength subtractive re-shaping of the few-layer MoS2 film into a one-dimensional (1D) nanostripe array results in a pronounced photonic anomaly, tunable in a broadband spectral range by simply changing the illumination conditions (or the lattice periodicity). This scheme promotes efficient coupling of light to the 2D TMD layers via resonant interaction between the MoS2 excitons and the photonic lattice, with subsequent enhancement of absorption exceeding 400% relative to the flat layer. In parallel, an ultra-broadband absorption amplification in the whole visible spectrum is achieved, thanks to the non-resonant excitation of substrate guided modes …
Royal Society of Chemistry
Publication date: 
1 Jan 2020

Mukul Bhatnagar, Maria Caterina Giordano, Carlo Mennucci, Debasree Chowdhury, Andrea Mazzanti, Giuseppe Della Valle, Christian Martella, Pinakapani Tummala, Alessio Lamperti, Alessandro Molle, Francesco Buatier de Mongeot

Biblio References: 
Volume: 12 Issue: 48 Pages: 24385-24393